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Free, publicly-accessible full text available March 11, 2026
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Kim, Gwangwoo; Huet, Benjamin; Stevens, Christopher E; Jo, Kiyoung; Tsai, Jeng-Yuan; Bachu, Saiphaneendra; Leger, Meghan; Song, Seunguk; Rahaman, Mahfujur; Ma, Kyung Yeol; et al (, Nature Communications)Abstract Two-dimensional (2D) semiconductors are promising candidates for optoelectronic application and quantum information processes due to their inherent out-of-plane 2D confinement. In addition, they offer the possibility of achieving low-dimensional in-plane exciton confinement, similar to zero-dimensional quantum dots, with intriguing optical and electronic properties via strain or composition engineering. However, realizing such laterally confined 2D monolayers and systematically controlling size-dependent optical properties remain significant challenges. Here, we report the observation of lateral confinement of excitons in epitaxially grown in-plane MoSe2quantum dots (~15-60 nm wide) inside a continuous matrix of WSe2monolayer film via a sequential epitaxial growth process. Various optical spectroscopy techniques reveal the size-dependent exciton confinement in the MoSe2monolayer quantum dots with exciton blue shift (12-40 meV) at a low temperature as compared to continuous monolayer MoSe2. Finally, single-photon emission (g2(0) ~ 0.4) was also observed from the smallest dots at 1.6 K. Our study opens the door to compositionally engineered, tunable, in-plane quantum light sources in 2D semiconductors.more » « lessFree, publicly-accessible full text available December 1, 2025
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Kim, Kwan-Ho; Song, Seunguk; Kim, Bumho; Musavigharavi, Pariasadat; Trainor, Nicholas; Katti, Keshava; Chen, Chen; Kumari, Shalini; Zheng, Jeffrey; Redwing, Joan M.; et al (, ACS Nano)
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Kim, Kwan-Ho; Oh, Seyong; Fiagbenu, Merrilyn Mercy; Zheng, Jeffrey; Musavigharavi, Pariasadat; Kumar, Pawan; Trainor, Nicholas; Aljarb, Areej; Wan, Yi; Kim, Hyong Min; et al (, Nature Nanotechnology)
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